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The legendary Pokemon you can catch in Pokemon Pearl are; Uxie Azelf Mesprit Palkia Heatran Regigigas (Regirock, Registeel and Regice are required) Giratina Cresselia Darkrai (requires Member Card) Shaymin (requires Oak's Letter) Arceus (requires Azure Flute)
The rest can be traded from other games, but not caught.